eprintid: 10112351 rev_number: 15 eprint_status: archive userid: 608 dir: disk0/10/11/23/51 datestamp: 2020-10-15 12:34:55 lastmod: 2021-09-26 23:19:13 status_changed: 2020-10-15 12:34:55 type: article metadata_visibility: show creators_name: Wu, C creators_name: Yu, G creators_name: Yin, Y creators_name: Wang, Y creators_name: Chen, L creators_name: Han, Q creators_name: Tang, J creators_name: Wang, B title: Mesoporous Polymeric Cyanamide-Triazole-Heptazine Photocatalysts for Highly-Efficient Water Splitting ispublished: pub divisions: UCL divisions: B04 divisions: C05 divisions: F43 keywords: conjugated polymers, hydrogen evolution reaction, oxygen evolution reaction, photocatalysts, water splitting note: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions. abstract: Conjugated polymers are promising light harvesters for water reduction/oxidation due to their simple synthesis and adjustable bandgap. Herein, both cyanamide and triazole functional groups are first incorporated into a heptazine‐based carbon nitride (CN) polymer, resulting in a mesoporous conjugated cyanamide‐triazole‐heptazine polymer (CTHP) with different compositions by increasing the quantity of cyanamide/triazole units in the CN backbone. Varying the compositions of CTHP modulates its electronic structures, mesoporous morphologies, and redox energies, resulting in a significantly improved photocatalytic performance for both H2 and O2 evolution under visible light irradiation. A remarkable H2 evolution rate of 12723 µmol h−1 g−1 is observed, resulting in a high apparent quantum yield of 11.97% at 400 nm. In parallel, the optimized photocatalyst also exhibits an O2 evolution rate of 221 µmol h−1 g−1, 9.6 times higher than the CN counterpart, with the value being the highest among the reported CN‐based bifunctional photocatalysts. This work provides an efficient molecular engineering approach for the rational design of functional polymeric photocatalysts. date: 2020-08-12 date_type: published publisher: WILEY-V C H VERLAG GMBH official_url: http://dx.doi.org/10.1002/smll.202003162 oa_status: green full_text_type: other language: eng primo: open primo_central: open_green verified: verified_manual elements_id: 1808230 doi: 10.1002/smll.202003162 lyricists_name: Tang, Junwang lyricists_id: JTANG13 actors_name: Tang, Junwang actors_id: JTANG13 actors_role: owner full_text_status: public publication: Small volume: 16 number: 37 pages: 9 citation: Wu, C; Yu, G; Yin, Y; Wang, Y; Chen, L; Han, Q; Tang, J; Wu, C; Yu, G; Yin, Y; Wang, Y; Chen, L; Han, Q; Tang, J; Wang, B; - view fewer <#> (2020) Mesoporous Polymeric Cyanamide-Triazole-Heptazine Photocatalysts for Highly-Efficient Water Splitting. Small , 16 (37) 10.1002/smll.202003162 <https://doi.org/10.1002/smll.202003162>. Green open access document_url: https://discovery-pp.ucl.ac.uk/id/eprint/10112351/1/fianl.pdf