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Frustrated Ising chains on the triangular lattice in Sr3NiIrO6

Toth, S; Wu, W; Adroja, DT; Rayaprol, S; Sampathkumaran, EV; (2016) Frustrated Ising chains on the triangular lattice in Sr3NiIrO6. Physical Review B , 93 , Article 174422. 10.1103/PhysRevB.93.174422. Green open access

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Abstract

Inelastic neutron scattering study on the spin-chain compound Sr3NiIrO6 reveals gapped quasi-1D magnetic excitations. The observed one-magnon band between 29.5 and 39 meV consists of magnon modes of the Ni2+ ions. The fitting of the spin wave spectrum reveals strongly coupled Ising-like chains along the c axis that are weakly coupled into a frustrated triangular lattice in the ab plane. The magnetic excitations survive up to 200 K well above the magnetic ordering temperature of TN ∼ 75 K, also indicating a quasi-1D nature of the magnetic interactions in Sr3NiIrO6. Our microscopic model is in agreement with ab initio electronic structure calculations and explains the giant spin-flip field observed in bulk magnetization measurements.

Type: Article
Title: Frustrated Ising chains on the triangular lattice in Sr3NiIrO6
Open access status: An open access version is available from UCL Discovery
DOI: 10.1103/PhysRevB.93.174422
Publisher version: https://doi.org/10.1103/PhysRevB.93.174422
Language: English
Additional information: This version is the version of record. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Science & Technology, Physical Sciences, Physics, Condensed Matter, Physics, COMPOUND, CA3CO2O6, TRANSITIONS, CSCOBR3, NET
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > MAPS Faculty Office
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > MAPS Faculty Office > Institute for Materials Discovery
URI: https://discovery-pp.ucl.ac.uk/id/eprint/10044075
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