Negahdar, L;
Parlett, C;
Isaacs, MA;
Beale, AM;
Wilson, K;
Lee, AF;
(2020)
Shining light on the solid-liquid interface: in-situ/operando monitoring of surface catalysis.
Catalysis Science & Technology
10.1039/d0cy00555j.
(In press).
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Abstract
Many industrially important chemical transformations occur at the interface between a solid catalyst and liquid reactants, despite which relatively little attention has been paid to spectroscopic methods for interrogating the working solid–liquid interface. This partly reflects a limited number of analytical techniques that give access to interface-specific information. Direct observation of surface species at catalytic solid–liquid interfaces is a daunting challenge for many in situ techniques due to the low concentration and/or short lifetime of chemical species in dynamic reactions. This review discusses the application of in situ and operando spectroscopies to probe solid–liquid interfaces, with a focus on the resulting mechanistic insight in the context of catalysis for sustainable chemistry.
| Type: | Article |
|---|---|
| Title: | Shining light on the solid-liquid interface: in-situ/operando monitoring of surface catalysis |
| Open access status: | An open access version is available from UCL Discovery |
| DOI: | 10.1039/d0cy00555j |
| Publisher version: | https://doi.org/10.1039/d0cy00555j |
| Language: | English |
| Additional information: | This article is licensed under a Creative Commons Attribution-NonCommercial 3.0 Unported Licence. http://creativecommons.org/licenses/by-nc/3.0/ |
| UCL classification: | UCL UCL > Provost and Vice Provost Offices > UCL BEAMS UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry |
| URI: | https://discovery-pp.ucl.ac.uk/id/eprint/10101141 |
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