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Molecular Auger Interferometry

Khokhlova, M; Cooper, B; Ueda, K; Prince, KC; Kolorenč, P; Ivanov, M; Averbukh, V; (2020) Molecular Auger Interferometry. In: Journal of Physics: Conference Series. IOP Publishing Green open access

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Abstract

We propose a theory of interferometric measurement of a normal Auger decay width in molecules. Molecular Auger interferometry is based on the coherent phase control of Auger dynamics in a two-colour (ω/2ω) laser field. We show that, in contrast to atoms, in oriented molecules of certain point groups (e.g. CH3F) the relative ω/2ω phase modulates the total ionisation yield. A simple analytical formula is derived for the extraction of the widths of Auger-active states from a molecular Auger interferogram, avoiding the need of either attosecond or high-resolution spectroscopy.

Type: Proceedings paper
Title: Molecular Auger Interferometry
Event: 31st International Conference on Photonic, Electronic and Atomic Collisions (ICPEAC XXXI)
Open access status: An open access version is available from UCL Discovery
DOI: 10.1088/1742-6596/1412/13/132001
Publisher version: https://doi.org/10.1088/1742-6596/1412/13/132001
Language: English
Additional information: © 2020 IOP Publishing. Content from this work may be used under the terms of theCreative Commons Attribution 3.0 licence (http://creativecommons.org/licenses/by/3.0).
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Physics and Astronomy
URI: https://discovery-pp.ucl.ac.uk/id/eprint/10106778
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