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Oxy-fuel Combustion for Carbon Capture and Sequestration (CCS) from a Coal/Biomass Power Plant: Experimental and Simulation Studies

Jurado Pontes, N; Darabkhani, H; Anthony, EJ; Oakey, J; (2014) Oxy-fuel Combustion for Carbon Capture and Sequestration (CCS) from a Coal/Biomass Power Plant: Experimental and Simulation Studies. Progress in Clean Energy , 2 pp. 177-192. 10.1007/978-3-319-17031-2_14. Green open access

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Abstract

Oxy-fuel combustion is a promising and relatively new technology to facilitate CO2 capture and sequestration (CCS) for power plants utilising hydrocarbon fuels. In this research experimental oxy-combustion trials and simulation are carried out by firing pulverised coal and biomass and co-firing a mixture of them in a 100 kW retrofitted oxy-combustor at Cranfield University. The parent fuels are coal (Daw Mill) and biomass cereal co-product (CCP) and experimental work was done for 100 % coal (w/w), 100 % biomass (w/w) and a blend of coal 50 % (w/w) and biomass 50 % (w/w). The recirculation flue gas (RFG) rate was set at 52 % of the total flue gas. The maximum percentage of CO2 observed was 56.7 % wet basis (73.6 % on a dry basis) when 100 % Daw Mill coal was fired. Major and minor emission species and gas temperature profiles were obtained and analysed for different fuel mixtures. A drop in the maximum temperature of more than 200 K was observed when changing the fuel from 100 % Daw Mill coal to 100 % cereal co-product biomass. Deposits formed on the ash deposition probes were also collected and analysed using the environmental scanning electron microscopy (ESEM) with energy-dispersive X-ray (EDX) technique. The high sulphur, potassium and chlorine contents detected in the ash generated using 100 % cereal co-product biomass are expected to increase the corrosion potential of these deposits. In addition, a rate-based simulation model has been developed using Aspen Plus® and experimentally validated. It is concluded that the model provides an adequate prediction for the gas composition of the flue gas.

Type: Article
Title: Oxy-fuel Combustion for Carbon Capture and Sequestration (CCS) from a Coal/Biomass Power Plant: Experimental and Simulation Studies
Open access status: An open access version is available from UCL Discovery
DOI: 10.1007/978-3-319-17031-2_14
Publisher version: https://doi.org/10.1007/978-3-319-17031-2_14
Language: English
Additional information: This version is the author accepted manuscript. For information on re-use, please refer to the publisher’s terms and conditions.
Keywords: Oxy-fuel combustion, Carbon capture and sequestration (CCS), Co-firing coal and biomass, Process modelling
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Mechanical Engineering
URI: https://discovery-pp.ucl.ac.uk/id/eprint/10117394
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