Gonzalez-Juarez, Maria de Lourdes;
Isaacs, Mark A;
Bradshaw, Darren;
Nandhakumar, Iris;
(2023)
Enhanced Thermoelectric Properties of a Semiconducting Two-Dimensional Metal–Organic Framework via Iodine Loading.
ACS Applied Materials and Interfaces
, 15
(4)
pp. 5478-5486.
10.1021/acsami.2c20770.
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Abstract
We report the first result of a study in which molecular iodine has been incorporated via incipient wetness impregnation into the two-dimensional semiconducting metal–organic framework (MOF) Cu3(2,3,6,7,10,11-hexahydroxytriphenylene)2 Cu3(HHTP)2 to enhance its thermoelectric properties. A power factor of 0.757 μW m–1 K–2 for this MOF was obtained which demonstrates that this provides an effective route for the preparation of moderate-performance thermoelectric MOFs.
| Type: | Article |
|---|---|
| Title: | Enhanced Thermoelectric Properties of a Semiconducting Two-Dimensional Metal–Organic Framework via Iodine Loading |
| Open access status: | An open access version is available from UCL Discovery |
| DOI: | 10.1021/acsami.2c20770 |
| Publisher version: | https://doi.org/10.1021/acsami.2c20770 |
| Language: | English |
| Additional information: | © 2023 The Authors. Published by American Chemical Society. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/), which permits unrestricted use, distribution, and reproduction in any medium, provided the original work is properly cited. |
| Keywords: | conducting metal−organic frameworks dip coating iodine thermoelectrics |
| UCL classification: | UCL UCL > Provost and Vice Provost Offices > UCL BEAMS UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry |
| URI: | https://discovery-pp.ucl.ac.uk/id/eprint/10164225 |
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