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N, S co-doped porous graphene-like carbon synthesized by a facile coal tar pitch-blowing strategy for high-performance supercapacitors

Li, Gang; Chen, Shanshan; Wang, Yonggang; Wang, Gang; Wu, Yuhan; Xu, Yang; (2023) N, S co-doped porous graphene-like carbon synthesized by a facile coal tar pitch-blowing strategy for high-performance supercapacitors. Chemical Physics Letters , 827 , Article 140712. 10.1016/j.cplett.2023.140712. Green open access

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Abstract

Herein, coal tar pitch (CTP) derived nitrogen and sulfur co-doped porous graphene-like carbon (NSPC) is performed by an ammonium sulfate-assisted chemical blowing strategy. Afterward, NSPC was activated by KOH to form a-NSPC features a bubble-like structure with a thin porous shell and a well-balanced porous ratio. Serving as electrode materials for supercapacitors, the capacitance of a-NSPC was 368 F g−1 at 0.5 A g−1. Meanwhile, the prepared materials exhibit excellent cycling stability after 10,000 cycles. This work may not only prepare superior electrode materials but also provide a feasible strategy for large-scale production of high-performance and low-cost electrode materials.

Type: Article
Title: N, S co-doped porous graphene-like carbon synthesized by a facile coal tar pitch-blowing strategy for high-performance supercapacitors
Open access status: An open access version is available from UCL Discovery
DOI: 10.1016/j.cplett.2023.140712
Publisher version: https://doi.org/10.1016/j.cplett.2023.140712
Language: English
Additional information: © 2023 The Author(s). Published by Elsevier B.V. This is an open access article under the CC BY license (http://creativecommons.org/licenses/by/4.0/).
Keywords: Coal tar pitch, Heteroatom doping, Graphene-like carbon, Blowing strategy, Supercapacitor
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Maths and Physical Sciences > Dept of Chemistry
URI: https://discovery-pp.ucl.ac.uk/id/eprint/10173663
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