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Facile synthesis: from Laminaria hyperborea to cellulose films and fibers

Dai, Yanqi; Sun, Dongyang; Sundaram, Senthilarasu; Delbusso, Angelo; O’Rourke, Dominic; Dorris, Mark; Edirisinghe, Mohan; (2023) Facile synthesis: from Laminaria hyperborea to cellulose films and fibers. Cellulose 10.1007/s10570-023-05606-w. (In press). Green open access

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Abstract

Inverted nozzle-pressurized gyration was used as a processing methodology for regenerating cellulose extracted from Laminaria hyperborea for the first time. The viscoelasticity of cellulose/1-ethyl-3-methylimidazolium acetate (EMIM OAc) solutions exhibited high concentration dependence, leading to the production of cellulose products with diverse structures. The regenerated cellulose transitioned from thin films to fibers (≈ 5 μm diameter) as the concentration was increased. The impact of collection distance and working pressure on the morphology and yield of fibers was investigated. This work provides a new sustainable route for processing biopolymers, offering significant potential for applications in biomedicine and healthcare.

Type: Article
Title: Facile synthesis: from Laminaria hyperborea to cellulose films and fibers
Open access status: An open access version is available from UCL Discovery
DOI: 10.1007/s10570-023-05606-w
Publisher version: http://dx.doi.org/10.1007/s10570-023-05606-w
Language: English
Additional information: This article is licensed under a Creative Commons Attribution 4.0 International License, which permits use, sharing, adaptation, distribution and reproduction in any medium or format, as long as you give appropriate credit to the original author(s) and the source, provide a link to the Creative Commons licence, and indicate if changes were made. The images or other third party material in this article are included in the article's Creative Commons licence, unless indicated otherwise in a credit line to the material. If material is not included in the article's Creative Commons licence and your intended use is not permitted by statutory regulation or exceeds the permitted use, you will need to obtain permission directly from the copyright holder. To view a copy of this licence, visit http://creativecommons.org/licenses/by/4.0/.
Keywords: Cellulose; Fibers; Pressurized gyration; Biopolymers; Sustainability
UCL classification: UCL
UCL > Provost and Vice Provost Offices > UCL BEAMS
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science
UCL > Provost and Vice Provost Offices > UCL BEAMS > Faculty of Engineering Science > Dept of Mechanical Engineering
URI: https://discovery-pp.ucl.ac.uk/id/eprint/10184350
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